Barcroft is a neighborhood in Arlington, Virginia with a population of 3,865. Barcroft is in Arlington County and is one of the best places to live in Virginia. In Barcroft, most residents own their homes. In Barcroft, there are a lot of restaurants, coffee shops, and parks. Many families and young professionals live in Barcroft and residents tend to be liberal. The public schools in Barcroft are highly rated.